A representation of the machine learning approach used to classify sulfur-38 nuclei (38S) from all other nuclei created in a complex nuclear reaction (left) and the resulting ability to gain knowledge of the unique sulfur-38 quantum "fingerprint" (right). Credit: Argonne National Laboratory

Fixed numbers of protons and neutrons—the building blocks of nuclei—can rearrange themselves within a single nucleus. The products of this reshuffling include electromagnetic (gamma ray) transitions. These transitions connect excited energy levels called quantum levels, and the pattern in these connections provide a unique "fingerprint" for each isotope.

Determining these fingerprints provides a sensitive test of scientists' ability to describe one of the , the strong (nuclear) force that holds protons and neutrons together.

In the laboratory, scientists can initiate the movement of protons and neutrons through an injection of excess using a nuclear reaction.

published in Âé¶¹ÒùÔºical Review C, researchers successfully used this approach to study the fingerprint of sulfur-38. They also used machine learning and other cutting-edge tools to analyze the data.

The results provide new empirical information on the "fingerprint" of quantum energy levels in the sulfur-38 nucleus. Comparisons with may lead to important new insights. For example, one of the calculations highlighted the key role played by a particular nucleon orbital in the model's ability to reproduce the fingerprints of sulfur-38 as well as neighboring nuclei.

The study is also important for its first successful implementation of a specific machine learning-based approach to classifying data. Scientists are adopting this approach to other challenges in .

Researchers used a measurement that included a (ML) assisted analysis of the collected data to better determine the unique quantum energy levels—a "fingerprint" formed through the rearrangement of the protons and neutrons—in the neutron-rich nucleus sulfur-38.

The results doubled the amount of empirical information on this particular fingerprint. They used a nuclear reaction involving the fusion of two nuclei, one from a heavy-ion beam and the second from a target, to produce the isotope and introduce the energy needed to excite it into higher quantum levels.

The reaction and measurement leveraged a heavy-ion beam produced by the ATLAS Facility (a Department of Energy user facility), a target produced by the Center for Accelerator and Target Science (CATS), the detection of electromagnetic decays (gamma-rays) using the , and the detection of the nuclei produced using the .

Due to complexities in the experimental parameters—which hinged between the production yields of the sulfur-38 nuclei in the reaction and the optimal settings for detection—the research adapted and implemented ML techniques throughout the data reduction.

These techniques achieved significant improvements over other techniques. The ML-framework itself consisted of a fully connected neural network that was trained under supervision to classify sulfur-38 nuclei against all other isotopes produced by the .

More information: C. R. Hoffman et al, Experimental study of the 38S excited level scheme, Âé¶¹ÒùÔºical Review C (2023). . On arXiv (2023):